Was the de-polarization of tariffs after Smoot-Hawley and WWII part of what allowed the Buckeyite wing of the GOP to form?
What it did do was remove the glue that held the GOP coalition together. Just as free trade, immigration and business regulation had always unified the Democrats for the most part, protectionism had been the unifier for the GOP like tax cuts are today. Not only did it keep progressive and conservative Republicans under the same nationalist roof, but it also got working class voters to support a coalition dominated by yankee business elites.
Once the tariff was removed as a legitimate policy tool, urban GOP machines began to collapse, because that was what kept the workers under the same roof. At the same time the GOP lost the workers, they also lost the African American urban vote to the New Deal coalition as well. This meant that the politically neutered middle and upper middle class whites who had previous dominated large segments of urban America, began to move to the Suburbs or move South.
Smoot-Hawley is important thus as one of many factors that tore apart the old GOP hegemony of the North and forced it to look South and West for new outlets of support.